Weak-Field, Multiple-Cycle Carrier Envelope Phase Effects in Laser Excitation

Klaus Renziehausen, Kilian Hader, Werner Jakubetz, Volker Engel (Korresp. Autor*in)

Veröffentlichungen: Beitrag in FachzeitschriftArtikelPeer Reviewed


Although the absolute or carrier envelope phase (CEP) of a laser pulse is usually assumed to be effective for ultrashort and/or ultrastrong pulses only, it is demonstrated that these limitations can eventually be removed. Therefore, the excitation of a model positively charged homonuclear diatomic molecule, in which four electronic states are coupled by the laser field, is studied. In an initial step, nuclear wave packets in two dissociative states are prepared. Upon reaching the fragment channel, a weak pulse interacts with the system and prepares CEP-dependent asymmetries associated with electron density localized on one or the other fragmentation product.
Seiten (von - bis)1464-1470
FachzeitschriftChemPhysChem: a European journal of chemical physics and physical chemistry
AusgabenummerSI 7
PublikationsstatusVeröffentlicht - 2013

ÖFOS 2012

  • 104017 Physikalische Chemie