An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds

Charles E. Kolb; R. Anthony Cox; Jonathan P D Abbatt; Markus Ammann; E. James Davis; D.J. Donaldson; Bruce C. Garrett; C. George; T. Griffiths; David R. Hanson; Markku Kulmala; Gordon B. McFiggans; Ulrich Pöschl; I Riipinen; Michel J. Rossi; Yinon Rudich; Paul Wagner; Paul Winkler; Douglas R. Worsnop; Colin O'Dowd

doi:10.5194/acp-10-10561-2010

An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds

Charles E. Kolb, R. Anthony Cox, Jonathan P D Abbatt, Markus Ammann, E. James Davis, D.J. Donaldson, Bruce C. Garrett, C. George, T. Griffiths, David R. Hanson, Markku Kulmala, Gordon B. McFiggans, Ulrich Pöschl, I Riipinen, Michel J. Rossi, Yinon Rudich, Paul Wagner, Paul Winkler, Douglas R. Worsnop, Colin O'Dowd

Aerosol Physics and Environmental Physics

Publications: Contribution to journal › Article › Peer Reviewed

Abstract

A workshop was held in the framework of the ACCENT (Atmospheric Composition Change – a European Network) Joint Research Programme on "Aerosols" and the Programme on "Access to Laboratory Data". The aim of the workshop was to hold "Gordon Conference" type discussion covering accommodation and reactive uptake of water vapour and trace pollutant gases on condensed phase atmospheric materials. The scope was to review and define the current state of knowledge of accommodation coefficients for water vapour on water droplet and ice surfaces, and uptake of trace gas species on a variety of different surfaces characteristic of the atmospheric condensed phase particulate matter and cloud droplets. Twenty-six scientists participated in this meeting through presentations, discussions and the development of a consensus review.

In this review we present an analysis of the state of knowledge on the thermal and mass accommodation coefficient for water vapour on aqueous droplets and ice and a survey of current state-of the-art of reactive uptake of trace gases on a range of liquid and solid atmospheric droplets and particles. The review recommends consistent definitions of the various parameters that are needed for quantitative representation of the range of gas/condensed surface kinetic processes important for the atmosphere and identifies topics that require additional research.

Original language	English
Pages (from-to)	10561-10605
Number of pages	45
Journal	Atmospheric Chemistry and Physics
Volume	10
Issue number	21
DOIs	https://doi.org/10.5194/acp-10-10561-2010
Publication status	Published - 2010

Austrian Fields of Science 2012

104017 Physical chemistry
103020 Surface physics
105904 Environmental research

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Kolb, C. E., Cox, R. A., Abbatt, J. P. D., Ammann, M., Davis, E. J., Donaldson, D. J., Garrett, B. C., George, C., Griffiths, T., Hanson, D. R., Kulmala, M., McFiggans, G. B., Pöschl, U., Riipinen, I., Rossi, M. J., Rudich, Y., Wagner, P., Winkler, P., Worsnop, D. R., & O'Dowd, C. (2010). An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds. Atmospheric Chemistry and Physics, 10(21), 10561-10605. https://doi.org/10.5194/acp-10-10561-2010

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Kolb, CE, Cox, RA, Abbatt, JPD, Ammann, M, Davis, EJ, Donaldson, DJ, Garrett, BC, George, C, Griffiths, T, Hanson, DR, Kulmala, M, McFiggans, GB, Pöschl, U, Riipinen, I, Rossi, MJ, Rudich, Y, Wagner, P, Winkler, P, Worsnop, DR & O'Dowd, C 2010, 'An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds', Atmospheric Chemistry and Physics, vol. 10, no. 21, pp. 10561-10605. https://doi.org/10.5194/acp-10-10561-2010

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AU - Donaldson, D.J.

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AU - Wagner, Paul

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AB - A workshop was held in the framework of the ACCENT (Atmospheric Composition Change – a European Network) Joint Research Programme on "Aerosols" and the Programme on "Access to Laboratory Data". The aim of the workshop was to hold "Gordon Conference" type discussion covering accommodation and reactive uptake of water vapour and trace pollutant gases on condensed phase atmospheric materials. The scope was to review and define the current state of knowledge of accommodation coefficients for water vapour on water droplet and ice surfaces, and uptake of trace gas species on a variety of different surfaces characteristic of the atmospheric condensed phase particulate matter and cloud droplets. Twenty-six scientists participated in this meeting through presentations, discussions and the development of a consensus review.In this review we present an analysis of the state of knowledge on the thermal and mass accommodation coefficient for water vapour on aqueous droplets and ice and a survey of current state-of the-art of reactive uptake of trace gases on a range of liquid and solid atmospheric droplets and particles. The review recommends consistent definitions of the various parameters that are needed for quantitative representation of the range of gas/condensed surface kinetic processes important for the atmosphere and identifies topics that require additional research.

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JO - Atmospheric Chemistry and Physics

JF - Atmospheric Chemistry and Physics

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ER -

An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds

Abstract

Austrian Fields of Science 2012

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