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Introduction to viscoelasticity and plasticity, and their relation to the underlying microscopic dynamics in soft matter systems

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Abstract

Understanding the rheological behavior of complex fluids, and in particular its relation to the dynamics of the elementary microscopic constituents, is one of the open challenges in soft matter science. In this contribution, we give a brief introduction to linear shear rheology and passive microrheology of soft amorphous materials, and we then focus on the transition to non-linearity during oscillatory rheology tests performed on soft glassy materials. These materials exhibit solid-like properties at rest, but they display characteristics of fluids when a sufficiently large shear is applied. Significant progress in understanding such ‘fluidization’ has been recently achieved by combining rheometry with techniques capable to capture the microscopic dynamics induced by shear, and in particular by oscillatory shear. We here summarize some of these achievements, as an introduction to the field for a non-expert reader.
Original languageEnglish
Article number128653
Number of pages13
JournalPhysica A: Statistical Mechanics and its Applications
Volume631
DOIs
Publication statusPublished - 1 Dec 2023

Funding

Open Access funding provided by University of Vienna. The authors thank Paolo Edera, Fabio Giavazzi, Nikos Kalafatakis, George Petekidis for useful discussions. VT acknowledges support from the Swiss National Science Foundation (Grant No. 200021_197340). Open Access funding provided by University of Vienna. The authors thank Paolo Edera, Fabio Giavazzi, Nikos Kalafatakis, George Petekidis for useful discussions. VT acknowledges support from the Swiss National Science Foundation (Grant No. 200021_197340 ).

Austrian Fields of Science 2012

  • 103015 Condensed matter
  • 103029 Statistical physics

Keywords

  • Large amplitude oscillatory shear
  • Microrheology
  • Non-linear rheology
  • Plastic rearrangements
  • Shear induced dynamics
  • Soft glassy materials
  • Yielding

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