On the analysis of lead objects in an attempt to determine their age

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Abstract

This paper reports on the materials analysis of a set of lead objects, commonly referred to as “the Jordan codices” in an attempt to shed some light on when they were manufactured. The codices are controversial, debate centring on whether they date to the early Christian period or are modern fakes. We report, for the first time, trace element analysis of samples from the lead codices as well as pieces of modern lead by PIXE and RBS to explore the trace element “fingerprint” of the metal used; the lead isotope composition by MC-ICP-MS can identify the geo location of the origin of the materials used; the alpha particle emission from the lead due to the presence of the 210Pb isotope; and the amount of helium that is trapped in the lead due to the radioactive decay of trace amounts of 238U and 232Th contained in the material − the (U + Th)/He age. No single technique is able to show conclusively that the objects are either modern or ancient. All four techniques suffer weaknesses, which prevent a definitive conclusion from being reached. However, there are indications that while some of the objects examined show signs of being contemporary, others appear to be older. It can be concluded that for some key examples we have been unable to show them to be made from contemporary materials and would suggest that this provides a good reason for scholars to treat the objects seriously and to perform further research on these objects.
Original languageEnglish
Article number165947
Number of pages11
JournalNuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
Volume570
DOIs
Publication statusPublished - Jan 2026

Funding

This project has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement No 824096 for the AMS work in Vienna and from the EPSRC NRF grant EP/X015491 for the Ion Beam Analysis work at Surrey. We thank the VERA team, especially Martin Martschini and Robin Golser, for help in AMS and inspiring discussions. We would also like to thank the British Geological Survey (BGS) team for their analysis of the lead isotopes at their ICP-MS facility and Chris Jeynes for his early efforts in the 210 Pb analysis of some of these samples. Also to Geoff Grime for discussions on the interpretation of the PIXE data and identification of ALL of the peaks due to Pb.

FundersFunder number
European Union824096
Electron Paramagnetic Resonance Spectroscopy National Research Facility (EPSRC NRF)EP/X015491

    Austrian Fields of Science 2012

    • 103014 Nuclear physics
    • 103012 High energy physics

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