Prediction of insulating quasicrystalline approximants using ab initio electronic structure calculations

Marian Krajci, Juergen Hafner

    Publications: Contribution to journalArticlePeer Reviewed

    Abstract

    Ab initio density-functional calculations have been used to search for icosahedral Al-transition-metal alloys with insulating behavior. We predict that low-order approximants to icosahedral AlPdTM, TM = Co, Rh, Ir are narrow-gap semiconductors. The stability of the gap suggests that it will survive in the quasicrystalline limit at least as a very deep pseudogap. We show that gap formation results from strong orbital hybridization and metallocovalent bonding, in analogy to many crystalline aluminides.
    Original languageEnglish
    Article number052201
    Number of pages4
    JournalPhysical Review B
    Volume67
    Issue number5
    DOIs
    Publication statusPublished - 2003

    Austrian Fields of Science 2012

    • 1030 Physics, Astronomy

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