Rapid cloud removal of dimethyl sulfide oxidation products limits SO2 and cloud condensation nuclei production in the marine atmosphere

Gordon A. Novak; Charles H. Fite; Christopher D. Holmes; Patrick R. Veres; J. Andrew Neuman; Ian Faloona; Joel A. Thornton; Glenn M. Wolfe; Michael P. Vermeuel; Christopher M. Jernigan; Jeff Peischl; Thomas B. Ryerson; Chelsea R. Thompson; Ilann Bourgeois; Carsten Warneke; Georgios I. Gkatzelis; Mathew M. Coggon; Kanako Sekimoto; T. Paul Bui; Jonathan Dean-Day; Glenn S. Diskin; Joshua P. DiGangi; John B. Nowak; Richard H. Moore; Elizabeth B. Wiggins; Edward L. Winstead; Claire Robinson; K. Lee Thornhill; Kevin J. Sanchez; Samuel R. Hall; Kirk Ullmann; Maximilian Dollner; Bernadett Weinzierl; Donald R. Blake; Timothy H. Bertram

doi:10.1073/pnas.2110472118

Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere

Gordon A. Novak
, Charles H. Fite
, Christopher D. Holmes
, Patrick R. Veres
, J. Andrew Neuman
, Ian Faloona
, Joel A. Thornton
, Glenn M. Wolfe
, Michael P. Vermeuel
, Christopher M. Jernigan
, Jeff Peischl
, Thomas B. Ryerson
, Chelsea R. Thompson
, Ilann Bourgeois
, Carsten Warneke
, Georgios I. Gkatzelis
, Mathew M. Coggon
, Kanako Sekimoto
, T. Paul Bui
, Jonathan Dean-Day

Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Richard H. Moore, Elizabeth B. Wiggins, Edward L. Winstead, Claire Robinson, K. Lee Thornhill, Kevin J. Sanchez, Samuel R. Hall, Kirk Ullmann, Maximilian Dollner, Bernadett Weinzierl, Donald R. Blake, Timothy H. Bertram (Corresponding author)

Aerosol Physics and Environmental Physics

Publications: Contribution to journal › Article › Peer Reviewed

Original language	English
Article number	e2110472118
Number of pages	7
Journal	Proceedings of the National Academy of Sciences of the United States of America
Volume	118
Issue number	42
Early online date	11 Oct 2021
DOIs	https://doi.org/10.1073/pnas.2110472118
Publication status	Published - 19 Oct 2021

Funding

ACKNOWLEDGMENTS. This work was supported by NSF Grant GEO AGS 1822420 and through the NSF Center for Aerosol Impacts on Chemistry of the Environment under Grant CHE 1801971. We would like to acknowledge the NASA Airborne Science Program and the NASA SARP. The authors also thank the SARP and ATom leadership and science teams and NASA DC-8 flight and ground crew for contributions to the measurements. C.H.F. and C.D.H. acknowledge support by the Future Investigators in NASA Earth and Space Science and Technology program (80NSSC19K1368) and NASA New Investigator Program (NNX16AI57G). The Langley Aerosol Research Group was supported by the NASA Tropospheric Chemistry Program (Dr. Barry Lefer, Program Manager). I.F. is supported by the California Agricultural Experiment Station funded by US Department of Agriculture, National Institute of Food and Agriculture Hatch project CA-D-LAW-2481-H. B.W. and M.D. would like to acknowledge funding from the European Research Council under the European Union’s Horizon 2020 research and innovation framework program under Grant Agreement No. 640458. We would like to acknowledge Zachary Finewax, Emmanuel Assaf, and James Burkholder at the National Oceanic and Atmospheric Administration Chemical Sciences Laboratory for their work in developing a quantitative method for HPMTF calibration.

Austrian Fields of Science 2012

103037 Environmental physics
103039 Aerosol physics
105208 Atmospheric chemistry

Keywords

Cloud condensation nuclei
Cloud processing
Dimethyl sulfide
Marine sulfur
Sulfate aerosol
marine sulfur
BOUNDARY-LAYER
dimethyl sulfide
sulfate aerosol
MECHANISM
SULFURIC-ACID
PARTICLE FORMATION
cloud processing
CHEMISTRY
cloud condensation nuclei
VOLATILE ORGANIC-COMPOUNDS

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1073/pnas.2110472118

Cite this

Novak, G. A., Fite, C. H., Holmes, C. D., Veres, P. R., Neuman, J. A., Faloona, I., Thornton, J. A., Wolfe, G. M., Vermeuel, M. P., Jernigan, C. M., Peischl, J., Ryerson, T. B., Thompson, C. R., Bourgeois, I., Warneke, C., Gkatzelis, G. I., Coggon, M. M., Sekimoto, K., Bui, T. P., ... Bertram, T. H. (2021). Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere. Proceedings of the National Academy of Sciences of the United States of America, 118(42), Article e2110472118. https://doi.org/10.1073/pnas.2110472118

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title = "Rapid cloud removal of dimethyl sulfide oxidation products limits SO2 and cloud condensation nuclei production in the marine atmosphere",

keywords = "Cloud condensation nuclei, Cloud processing, Dimethyl sulfide, Marine sulfur, Sulfate aerosol, marine sulfur, BOUNDARY-LAYER, dimethyl sulfide, sulfate aerosol, MECHANISM, SULFURIC-ACID, PARTICLE FORMATION, cloud processing, CHEMISTRY, cloud condensation nuclei, VOLATILE ORGANIC-COMPOUNDS",

author = "Novak, \{Gordon A.\} and Fite, \{Charles H.\} and Holmes, \{Christopher D.\} and Veres, \{Patrick R.\} and Neuman, \{J. Andrew\} and Ian Faloona and Thornton, \{Joel A.\} and Wolfe, \{Glenn M.\} and Vermeuel, \{Michael P.\} and Jernigan, \{Christopher M.\} and Jeff Peischl and Ryerson, \{Thomas B.\} and Thompson, \{Chelsea R.\} and Ilann Bourgeois and Carsten Warneke and Gkatzelis, \{Georgios I.\} and Coggon, \{Mathew M.\} and Kanako Sekimoto and Bui, \{T. Paul\} and Jonathan Dean-Day and Diskin, \{Glenn S.\} and DiGangi, \{Joshua P.\} and Nowak, \{John B.\} and Moore, \{Richard H.\} and Wiggins, \{Elizabeth B.\} and Winstead, \{Edward L.\} and Claire Robinson and Thornhill, \{K. Lee\} and Sanchez, \{Kevin J.\} and Hall, \{Samuel R.\} and Kirk Ullmann and Maximilian Dollner and Bernadett Weinzierl and Blake, \{Donald R.\} and Bertram, \{Timothy H.\}",

year = "2021",

month = oct,

day = "19",

doi = "10.1073/pnas.2110472118",

language = "English",

volume = "118",

journal = "Proceedings of the National Academy of Sciences of the United States of America",

issn = "0027-8424",

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Novak, GA, Fite, CH, Holmes, CD, Veres, PR, Neuman, JA, Faloona, I, Thornton, JA, Wolfe, GM, Vermeuel, MP, Jernigan, CM, Peischl, J, Ryerson, TB, Thompson, CR, Bourgeois, I, Warneke, C, Gkatzelis, GI, Coggon, MM, Sekimoto, K, Bui, TP, Dean-Day, J, Diskin, GS, DiGangi, JP, Nowak, JB, Moore, RH, Wiggins, EB, Winstead, EL, Robinson, C, Thornhill, KL, Sanchez, KJ, Hall, SR, Ullmann, K, Dollner, M , Weinzierl, B, Blake, DR & Bertram, TH 2021, 'Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere', Proceedings of the National Academy of Sciences of the United States of America, vol. 118, no. 42, e2110472118. https://doi.org/10.1073/pnas.2110472118

Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere. / Novak, Gordon A.; Fite, Charles H.; Holmes, Christopher D. et al.
In: Proceedings of the National Academy of Sciences of the United States of America, Vol. 118, No. 42, e2110472118, 19.10.2021.

Publications: Contribution to journal › Article › Peer Reviewed

TY - JOUR

T1 - Rapid cloud removal of dimethyl sulfide oxidation products limits SO2 and cloud condensation nuclei production in the marine atmosphere

AU - Novak, Gordon A.

AU - Fite, Charles H.

AU - Holmes, Christopher D.

AU - Veres, Patrick R.

AU - Neuman, J. Andrew

AU - Faloona, Ian

AU - Thornton, Joel A.

AU - Wolfe, Glenn M.

AU - Vermeuel, Michael P.

AU - Jernigan, Christopher M.

AU - Peischl, Jeff

AU - Ryerson, Thomas B.

AU - Thompson, Chelsea R.

AU - Bourgeois, Ilann

AU - Warneke, Carsten

AU - Gkatzelis, Georgios I.

AU - Coggon, Mathew M.

AU - Sekimoto, Kanako

AU - Bui, T. Paul

AU - Dean-Day, Jonathan

AU - Diskin, Glenn S.

AU - DiGangi, Joshua P.

AU - Nowak, John B.

AU - Moore, Richard H.

AU - Wiggins, Elizabeth B.

AU - Winstead, Edward L.

AU - Robinson, Claire

AU - Thornhill, K. Lee

AU - Sanchez, Kevin J.

AU - Hall, Samuel R.

AU - Ullmann, Kirk

AU - Dollner, Maximilian

AU - Weinzierl, Bernadett

AU - Blake, Donald R.

AU - Bertram, Timothy H.

PY - 2021/10/19

Y1 - 2021/10/19

KW - Cloud condensation nuclei

KW - Cloud processing

KW - Dimethyl sulfide

KW - Marine sulfur

KW - Sulfate aerosol

KW - marine sulfur

KW - BOUNDARY-LAYER

KW - dimethyl sulfide

KW - sulfate aerosol

KW - MECHANISM

KW - SULFURIC-ACID

KW - PARTICLE FORMATION

KW - cloud processing

KW - CHEMISTRY

KW - cloud condensation nuclei

KW - VOLATILE ORGANIC-COMPOUNDS

UR - https://www.scopus.com/pages/publications/85116912719

U2 - 10.1073/pnas.2110472118

DO - 10.1073/pnas.2110472118

M3 - Article

AN - SCOPUS:85116912719

SN - 0027-8424

VL - 118

JO - Proceedings of the National Academy of Sciences of the United States of America

JF - Proceedings of the National Academy of Sciences of the United States of America

IS - 42

M1 - e2110472118

ER -

Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere

Funding

Austrian Fields of Science 2012

Keywords

UN SDGs

Access to Document

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A-LIFE: Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics

Cite this

Rapid cloud removal of dimethyl sulfide oxidation products limits SO2 and cloud condensation nuclei production in the marine atmosphere

Funding

Austrian Fields of Science 2012

Keywords

UN SDGs

Access to Document

Other files and links

Fingerprint

Projects

A-LIFE: Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics

Cite this

Rapid cloud removal of dimethyl sulfide oxidation products limits SO₂ and cloud condensation nuclei production in the marine atmosphere